JLU-PERS Group
Plasmon-enhanced Raman spectroscopy (PERS)@Jilin University
表面等离子体光子学和表面增强光谱学研究的对象一般是光、分子和金属纳米结构相互作用的复杂体系，涉及到物理学、化学、生命科学、材料科学和纳米科学等多个学科领域；而在传统学科如分子光谱学和表面科学以及新兴的学科如纳米光学中一般仅涉及到光、分子和纳米结构三者中的任意两者之间的相互作用。目前，以光、分子和纳米结构三者之间相互作用为基本科学问题以及所产生相关新现象的研究成为国际上的极具前瞻性和挑战性的重要领域
Plasmon-Enhanced Spectroscopy
表面增强光谱学包括表面增强拉曼散射(SERS)，表面增强二次谐波[i] [ii] [iii] [iv]（surface enhanced second-harmonic generation, SE-SHG)，表面增强红外光谱[v][vi](surface enhanced infrared spectroscopy, SEIRS)，表面增强荧光(surface-enhanced fluorescence, SEF) [vii] 以及表面增强和频 (surface-enhanced sum frequency generation SE-SFG) [viii] [ix] [x]。
[i] Chen, C. K.; de Castro, A. R. B.; Shen, Y. R.; Surface-Enhanced Second-Harmonic Generation, Phys. Rev. Lett., 1981, 46, 145-148.
[ii] Rogovin, D.; Shen, T. P.; Microparticle surface-enhanced second-harmonic generation, J. Opt. Soc. Am. B, 1988, 5, 1886-1889.
[iii] Stockman. M. I.; Bergman, D. J.; Anceau, C.; Brasselet, S.; Zyss, J.; Enhanced second-harmonic generation by metal surfaces with nanoscale roughness: Nanoscale dephasing, depolarization, and correlations, Phys. Rev. Lett., 2004, 92, 057402.
[iv] Li, K. R.; Li, X. T.; Stockman, M. I.; Bergman, D. J.; Surface plasmon amplification by stimulated emission in nanolenses, Phys. Rev. B, 2005, 71, 153401.
[v] Zhang, Z. J.; Imae, T.; Study of Surface-Enhanced Infrared Spectroscopy: 1. Dependence of the Enhancement on Thickness of Metal Island Films and Structure of Chemisorbed Molecules, J. Colloid. Interface Sci., 2001, 233, 99-106.
[vi] Jensen. T. R.; Van Duyne, R. P.; Johnson, S. A.; Maroni, V. A.; Surface-enhanced infrared spectroscopy: A comparison of metal island films with discrete and nondiscrete surface plasmons, Appl. Spectrosc., 2000, 54, 371-377.
[vii] Lakowicz. J. R.; Geddes, C. D.; Gryczynski, I.; Malicka, J.; Gryczynski, Z.; Aslan, K.; Lukomska, J.; Matveeva, E.; Zhang, J. A.; Badugu, R.; Huang, J.; Advances in surface-enhanced fluorescence, J. Fluoresc., 2004, 14, 425-441.
[viii] Bonn, M.; Ueba, H.; Wolf, M.; Theory of sum-frequency generation spectroscopy of adsorbed molecules using the density matrix method - broadband vibrational sum-frequency generation and applications, J Phys-Condens Mat., 2005, 17, S201-S220.
[ix] Alieva, E. V.; Knippels, G. M. H.; Kuzik, L. A.; Mattei, G.; Van der Meer, A. F. G.; Yakovlev. V. A.; Sum-frequency generation spectra of thin organic films on silver enhanced due to surface plasmon excitation, Phys.Status. Solidi. A, 1999, 175, 109-114.
[x] Balakin. A. V.; Bushuev, V. A.; Mantsyzov, B. I.; Ozheredov, I. A.; Petrov, E. V.; Shkurinov, A. P.; Masselin, P.; Mouret, G.; Enhancement of sum frequency generation near the photonic band gap edge under the quasiphase matching conditions, Phys. Rev. E, 2001, 63, 046609.